Research

Single-Atom Catalyst for Environmental Application

Nanotechnology has been the main driver of scientific advances in catalytic materials and processes over the past few decades. Unique physicochemical and electronic properties emerge as materials are engineered from the large bulk to the nanoscale. What would happen if the same material were engineered to be even smaller and sub-nanoscale? Can the material be engineered to exist as a ‘single atom?’ Our group has been pioneering the synthesis and environmental application of single-atom catalysts (SACs), the theoretical limit of material downsizing. We target maximizing efficiency of atomic utilization due to size reduction from nanoscale catalysts, significantly reducing material and process costs, and achieving highly selective destruction of pollutant in complex water matrix which has been unable to address with nanotechnology.

Electrochemical Water Treatment

Electrochemical treatment is emerging as the next-generation technology to achieve modular, distributed, and chemical-free water treatment and recycling. Our group investigates various approaches to destroy a wide range of pollutants through both cathodic (e.g., reduction of oxyanions and halogenated organics including PFAS) and cathodic (e.g., direct oxidation and the production of reactive species) reactions. Our group develops various catalysts for electrodes including single-atom catalysts and fabricate electrochemical cells. We also study electrochemical synthesis of hydrogen peroxide, a precursor chemical for advanced oxidation.

Solar Water Disinfection in Developing Countries

Our group has been studying various approaches to provide affordable disinfection solution to resource-limited regions in the world. We have developed various next-generation technologies to harvest solar radiation to inactivate pathogens in water, including photosensitized water disinfection using food-dye and natural plant extracts, photothermal disinfection using plasmonic particles, and photocatalytic disinfection using various catalysts. We continue to explore different technologies, along with collaboration with various partners in the US and around the world for practical implementation.

Research Projects

Research
1. Precision Destruction of Organohalides by Single Atom Catalysts, NAWI, 2022-2025
2. Electrochemical Reclamation of Reverse Osmosis Concentrate, SK Innovation, 2021-2023
3. ERASE-PFAS: Collaborative Research: Nickel and Palladium Single-Atom Electrocatalysts for Selective Capture and Destruction of PFAS in Complex Water Matrices, National Science Foundation, 2021-2024
4. Solar Water Disinfection Window: From Light-Harvesting Material Development to Field Implementation, Engineering Research Center for Nanotechnology Enabled Water Treatment Systems (NEWT), 2020-2022
5. Solar Window for Water Collection and Purification, Environmental Protection Agency, 2020-2021
6. Environmental Materials Beyond and Below Nanoscale: Palladium Single Atom, National Science Foundation, 2020-2023
7. US-Israel Center of Excellence in Energy, Engineering and Water Technology, 2020-2025
8. Nanoparticle Enhanced Solar Photothermal Water Disinfection, NEWT, 2019-2020
9. Exploring Single Atom Catalyst for Water Treatment: Oxyanion Reduction, NEWT, 2018
10. Effective Destruction of Per- and Polyfluoroalkyl Substances in Water by Modified SiC-Based Photocatalysts, SERDP, 2018-2019
11. Self-healing Hydrogel-Composite Membranes: from Proof-of-Concept to Water Reuse Application, Water Environment & Reuse Foundation, 2018-2019
12. Photosensitizing Food Dyes for Water Treatment and Safety Indication, Amway Corporation, 2018
13. Quantifying the Disinfection Efficiency of Household UV Systems, Daelim Industrial, 2015-2016
14. Emerging Carbon-Based Nanomaterials in the Environment, Korea Institute of Toxicology, 2015-2016
15. Developing in-situ and Self-Healing Techniques for Water Treatment Membranes, Korea Institute of Advancement of Technology, 2014-2017 
16. Triplet-triplet Annihilation Upconversion in Silica Nanocapsules for Visible-Light Photocatalysis, Korea Institute of Industrial Technology, 2014
17. Upconversion Enhanced Visible Light Sensitization of Semiconductor Photocatalysts for Environmental Application, National Science Foundation, 2014-2017
18. Quantitative Insights on Environmental Implication of Functionalizing Fullerenes, National Science Foundation, 2012-2015
19. Optimizing Upconversion Phosphor Materials for Antimicrobial Surface Coating, Hwaseung T&C, 2011-2014
20. Converting Visible Light to UVC: Lanthanide Upconversion Nano-Phosphors for Light-Activated Biocidal Surface Development, National Science Foundation, 2011-2013